A study on optical characteristics of amorphous structure (Vitreous) including oxides of main and transitional elements in binary system B2O3 – CaO

Research Article

F. Ashrafi, S.A. Babanejad, A.

Abstract

Amorphous Structures have specific characteristics including semi-conductivity. Boron trioxide can form the vitreous structure with other oxides. Addition of certain oxides to boron trioxide modifies the properties of these glasses. In our investigation B2O3 - CaO binary was studies and it was appeared that the system of (100 – x) B2O3 – x CaO is able to form the vitreous structure and the range of x was determined experimentally. For better understanding the electronic structure and study on the edge-absorption, we can use optical absorption. By using a UV - Visible spectrophotometer the absorption spectrums were obtained. Studying these spectrums and by using Urbach and Mott-Davis theories, the absorption coefficient, α(ω), have calculated according to Bir-Lambert relation. By tracing (αħω)1/n against ħω plot, the amount of n was determined. For B2O3 - CaO binary system n = 1/2 was obtained. Extrapolating (αħω)2 against ħω plot, we can determine optical gap energy, Eopt , at (αħω)2 = 0. Obtaining results show that, Eopt increase with CaO percentage increasing. The coefficient B, also, is calculated by using Mott-Davis relation. By determining the slop of ln α(ω) against ħω diagram, the width of localized states in the energy of bonds, E, can be obtain

Relevant Publications in Der Chemica Sinica