A H-bonded Chloranilate Chain with an Unprecedented Topology

Samia Benmansour, Cristina Val

Abstract

New (PPh3Et)2(C6O4Cl2)·2H2O (1) compound has been synthetized and structurally characterized. This compound presents layers of cations and non coordinated [C6O4Cl4]2-anions alternating along thecdirection. The cationic layers contains isolated [PPh3Et]+ cations whereas in the anionic layers the chloranilate anions are connected forming chains along the a direction thanks to two H-bonds formed between the oxygen atoms of the chloranilate anions and two water molecules located between two anions. The topology of this H-bonded chain is unprecedented in any chloranilate compound. Compound 1 is the first characterized salt containing noncoordinated chloranilate anions with any phosphonium cation.

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